4,218 publications from this institution
Elevated temperature synthesis has been used to generate virtually defect free SiO2 sheathed crystalline silicon nanowires and silica (SiO2) nanospheres which can be agglomerated to wire-like configurations impregnated with crystalline silicon. The SiO2 passivated (sheathed) crystalline silicon nanowires, generated with a modified approach using a heated Si–SiO2 mix, with their axes parallel to 〈111〉 are found to be virtually defect free. Modifications to the system allow the simultaneous formation of SiO2 nanospheres (d∼10–30 nm) as virtually monodisperse gram quantity powders which form large surface area catalysts for the selective conversion of ethanol to acetaldehyde.
Rashba spin–orbit coupling (SOC) is a core issue in semiconductor spintronics, which allows the manipulation of electron spin through an electric field rather than an external magnetic field, revealing a bright prospect for advanced electronic devices with ultra-high speed and integration. Conversely, the emerging piezotronic effect is the born characteristic for many semiconductors that have a non-central symmetric structure, such as ZnO and GaN. Here, we design three heterostructure devices, based on piezoelectric p-type (CH3NH3)PbI3 single crystals and n-type wurtzite-structured ZnO thin films, to theoretically study how the piezotronic effect can effectively work on the Rashba spin–orbit coupling. Benefiting from large piezoelectric charges at the interface when a vertical strain is applied, a high concentration of two-dimensional electron gas is induced in the plane of the heterostructure, which can tune the built-in electric field at the interface and further manipulate the Rashba SOC. With the increase in pressure, both the Rashba parameter and spin splitting are found to first vanish and then increase linearly for ZnO with doping densities of 1015 and 1016 cm−3. This work provides insight for manipulating electron spins via the introduction of piezocharges, showing great application potential of the piezotronic effect in tuning spintronic devices.
Anisotropic growth in nanomaterials can lead to many interesting growth morphologies. This is especially true when the crystal structure contains anisotropy not only due to different surface plane energies but also due to surface polarity and/or chemical activity. Such is the case with wurtzite ZnS. This feature article covers the ZnS one-dimensional nanostructures that have been synthesized by a vapor–solid process, focusing on nanowires, nanorods, nanobelts, nanohelices and other derived nanostructures. This feature article mainly focuses on the polar surface dominated growth phenomena and the understanding of their formation mechanisms.
Designing, fabricating, and integrating arrays of nanodevices into a functional system are the key to transferring nanoscale science into applicable nanotechnology. We report large-array three-dimensional (3D) circuitry integration of piezotronic transistors based on vertical zinc oxide nanowires as an active taxel-addressable pressure/force sensor matrix for tactile imaging. Using the piezoelectric polarization charges created at a metal-semiconductor interface under strain to gate/modulate the transport process of local charge carriers, we designed independently addressable two-terminal transistor arrays, which convert mechanical stimuli applied to the devices into local electronic controlling signals. The device matrix can achieve shape-adaptive high-resolution tactile imaging and self-powered, multidimensional active sensing. The 3D piezotronic transistor array may have applications in human-electronics interfacing, smart skin, and micro- and nanoelectromechanical systems.
Journal Article Scanning Probe Microscopy in TEM : an In-situ Approach for Nano-scale Property Measurements Get access Zhong Lin (ZL) Wang Zhong Lin (ZL) Wang Center for Nanoscience and Nanotechnology, and School of Materials Science and Engineering, Georgia Institute of Technology, Atlanta, GA 30332-0245, e-mail: zhong.wang@mse.gatech.edu Search for other works by this author on: Oxford Academic Google Scholar Microscopy and Microanalysis, Volume 8, Issue S02, 1 August 2002, Pages 300–301, https://doi.org/10.1017/S1431927602100821 Published: 01 November 2002