Gate-tunable transmon qubits are based on quantum conductors used as weak links within hybrid Josephson junctions. These gatemons have been implemented in just a handful of systems, all relying on extended conductors, namely epitaxial semiconductors or exfoliated graphene. Here we present the coherent control of a gatemon based on a single molecule, a one-dimensional carbon nanotube, which is integrated into a circuit quantum electrodynamics architecture. The measured qubit spectrum can be tuned with a gate voltage and reflects the quantum dot behavior of the nanotube. Our ultraclean integration, using a hexagonal boron nitride substrate, results in record coherence times of 200 ns for carbon nanotube-based qubits. Furthermore, we investigate its decoherence mechanisms, thus revealing a strong gate dependence and identifying charge noise as a limiting factor. On top of positioning carbon nanotubes as contenders for future quantum technologies, our work paves the way for studying microscopic fermionic processes in low-dimensional quantum conductors.
Masiar Sistani, Jovian Delaforce, R. B. G. Kramer, Nicolas Roch, Minh Anh Luong, M. den Hertog, Éric Robin, J. Smoliner, Jun Yao, Charles M. Lieber, Cécile Naud, Alois Lugstein, O. Buisson
Masiar Sistani, Jovian Delaforce, R. B. G. Kramer, Nicolas Roch, Minh Anh Luong, M. den Hertog, Éric Robin, J. Smoliner, Jun Yao, Charles M. Lieber, Cécile Naud, Alois Lugstein, O. Buisson
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