Novel electrochemical behavior of silk protein to generate an adhesive electrogel is reported. The biomimetic system demonstrates reversible adhesive properties (see image) and functions on both hydrated and dry surfaces. Further, the system utilizes all-biocompatible components and functions in an all-aqueous process at ambient conditions. Potential applications in medical devices and in environmentally compatible material systems are described. Detailed facts of importance to specialist readers are published as "Supporting Information". Such documents are peer-reviewed, but not copy-edited or typeset. They are made available as submitted by the authors. Please note: The publisher is not responsible for the content or functionality of any supporting information supplied by the authors. Any queries (other than missing content) should be directed to the corresponding author for the article.
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