Effect of spin-dependent tunneling in a MoSe$_2$/Cr$_2$Ge$_2$Te$_6$ van der Waals heterostructure on exciton and trion emission — Annika Bergmann (2024) | RDL Network
Effect of spin-dependent tunneling in a MoSe$_2$/Cr$_2$Ge$_2$Te$_6$ van der Waals heterostructure on exciton and trion emission
Preprint 2024 en
Authors
AB
Annika Bergmann
SD
Swarup Deb
VS
Veronika Schneidt
Abstract
1 min read
We study van der Waals heterostructures consisting of monolayer MoSe$_2$ and few-layer Cr$_2$Ge$_2$Te$_6$ fully encapsulated in hexagonal Boron Nitride using low-temperature photoluminescence and polar magneto-optic Kerr effect measurements. Photoluminescence characterization reveals a partial quenching and a change of the exciton-trion emission ratio in the heterostructure as compared to the isolated MoSe$_2$ monolayer. Under circularly polarized excitation, we find that the exciton-trion emission ratio depends on the relative orientation of excitation helicity and Cr$_2$Ge$_2$Te$_6$ magnetization, even though the photoluminescence emission itself is unpolarized. This observation hints at an ultrafast, spin-dependent interlayer charge transfer that competes with exciton and trion formation and recombination.
T. P. Lyons, Daniel J. Gillard, Alejandro Molina‐Sánchez, Abhishek Misra, Freddie Withers, P. S. Keatley, Aleksey Kozikov, Takashi Taniguchi, Kenji Watanabe, Konstantin ‘kostya’ Novoselov, J. Fernández‐Rossier, A. I. Tartakovskii
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