Cementitious composites with recycled plastic often suffer from reduced strength. This study explores the partial substitution of cement with industrial by-products in plastic-based mortar mixes (PBMs) to enhance performance while reducing environmental impact. To achieve this, five hybrid machine learning (ML) models CNN-LSTM, XGBoost-PSO, SVM + K-Means, SVM-PSO, and XGBoost + K-Means were developed to predict flexural strength, production cost, and CO2 emissions using a large dataset compiled from peer-reviewed sources. The CNN-LSTM model consistently outperformed the other approaches, showing high predictive capability for both mechanical and sustainability-related outputs. Sensitivity analysis revealed that water content and superplasticizer dosage are the most influential factors in improving flexural strength, while excessive cement and plastic waste were found to negatively impact performance. The proposed ML framework was also successful in estimating production cost and CO2 emissions, demonstrating strong alignment between predicted and actual values. Beyond mechanical and environmental predictions, the framework was extended through the RA-PSO model to estimate compressive and tensile strengths with high reliability. To support practical adoption, the study proposes a graphical user interface (GUI) that allows engineers and researchers to efficiently evaluate durability, cost, and environmental indicators. In addition, the establishment of an open access data-sharing platform is recommended to encourage broader utilization of PBMs in the production of paving blocks and non-structural masonry units. Overall, this work highlights the potential of hybrid ML approaches to optimize sustainable cementitious composites, bridging the gap between performance requirements and environmental responsibility.
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