AC magnetometry of van der Waals magnets using ultrasensitive graphene Hall sensors

Abstract Probing the dynamical magnetic properties of two-dimensional (2D) materials requires sensitive techniques capable of detecting small magnetic fields from nanoscale samples. We demonstrate quantitative AC and DC magnetometry of a ferromagnetic Fe 3– x GeTe 2 nanoflakes using ultrasensitive graphene Hall sensors. These devices achieve record-low magnetic field detection noise at both cryogenic and room temperature, enabled by hexagonal boron nitride encapsulation, low-resistance fluorographene contacts, and a novel fabrication process. We perform quantitative AC susceptibility measurements up to 1 kHz, resolving both real and imaginary components with nanotesla-scale sensitivity and milliradian phase accuracy, the first such measurement in a van der Waals magnet. Our results establish graphene Hall sensors as a powerful and broadly applicable platform for studying magnetic and superconducting phases near the 2D limit.